Polarized and magic angle fifth-order 2D electronically non-resonant Raman scattering from CS2

David A. Blank, Laura J. Kaufman, Graham R. Fleming

Research output: Contribution to journalArticlepeer-review

Abstract

We have successfully used phase matching considerations to provide significant discrimination against cascaded lower-order responses and measured the direct fifth-order response from the intermolecular motions in liquid CS2. Here we report the measured polarized and magic angle responses and discuss comparisons with simulations.

Original languageEnglish (US)
Pages (from-to)513-515
Number of pages3
JournalSpringer Series in Chemical Physics
Volume66
DOIs
StatePublished - 2001

Bibliographical note

Funding Information:
Use of the Linac Coherent Light Source (LCLS) and the Stanford Synchrotron Radiation Lightsource (SSRL), SLAC National Accelerator Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences (contract No. DE-AC02-76SF00515). This study used resources from the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy (contract No. DE-AC02-05CH11231).

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