Nanoscale fluorescence lifetime imaging of an optical antenna with a single diamond NV center

Ryan Beams, Dallas Smith, Timothy W. Johnson, Sang Hyun Oh, Lukas Novotny, A. Nick Vamivakas

Research output: Contribution to journalArticlepeer-review

78 Scopus citations

Abstract

Solid-state quantum emitters, such as artificially engineered quantum dots or naturally occurring defects in solids, are being investigated for applications ranging from quantum information science and optoelectronics to biomedical imaging. Recently, these same systems have also been studied from the perspective of nanoscale metrology. In this letter, we study the near-field optical properties of a diamond nanocrystal hosting a single nitrogen vacancy center. We find that the nitrogen vacancy center is a sensitive probe of the surrounding electromagnetic mode structure. We exploit this sensitivity to demonstrate nanoscale fluorescence lifetime imaging microscopy (FLIM) with a single nitrogen vacancy center by imaging the local density of states of an optical antenna.

Original languageEnglish (US)
Pages (from-to)3807-3811
Number of pages5
JournalNano letters
Volume13
Issue number8
DOIs
StatePublished - Aug 14 2013

Keywords

  • NV center
  • Near-field scanning optical microscopy
  • fluorescence lifetime imaging
  • local density of optical states
  • optical antenna

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