Polarization-dependent detection of impulsive stimulated Raman scattering in α-quartz

Andy Rundquist; Jon Broman; David Underwood; David Blank

doi:10.1080/09500340500217415

Polarization-dependent detection of impulsive stimulated Raman scattering in α-quartz

Andy Rundquist, Jon Broman, David Underwood, David Blank

Chemistry (Twin Cities)

Research output: Contribution to journal › Article › peer-review

6 Scopus citations

Abstract

The stimulation and detection of both the A - and E -symmetry Raman lines in α-quartz using ultrafast impulsive stimulated Raman scattering is presented. Using a flexible experimental set-up, each nuclear oscillatory mode is selected and analysed in the time domain separately. The mode selection is made possible with optical summing of the fields involved to reduce noise and assure accurate synchronization. The experimental procedure is compared to optical heterodyne detection Raman-induced Kerr effect spectroscopy (OHD-RIKES) and the data is compared with standard frequency-domain measurements.

Original language	English (US)
Pages (from-to)	2501-2510
Number of pages	10
Journal	Journal of Modern Optics
Volume	52
Issue number	17
DOIs	https://doi.org/10.1080/09500340500217415
State	Published - Nov 20 2005

Bibliographical note

Funding Information:
The authors wish to thank Professor Guetter from Hamline University’s Mathematics Department and acknowledge support from the Research Corporation and the National Science Foundation.

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abstract = "The stimulation and detection of both the A - and E -symmetry Raman lines in α-quartz using ultrafast impulsive stimulated Raman scattering is presented. Using a flexible experimental set-up, each nuclear oscillatory mode is selected and analysed in the time domain separately. The mode selection is made possible with optical summing of the fields involved to reduce noise and assure accurate synchronization. The experimental procedure is compared to optical heterodyne detection Raman-induced Kerr effect spectroscopy (OHD-RIKES) and the data is compared with standard frequency-domain measurements.",

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AU - Underwood, David

AU - Blank, David

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N2 - The stimulation and detection of both the A - and E -symmetry Raman lines in α-quartz using ultrafast impulsive stimulated Raman scattering is presented. Using a flexible experimental set-up, each nuclear oscillatory mode is selected and analysed in the time domain separately. The mode selection is made possible with optical summing of the fields involved to reduce noise and assure accurate synchronization. The experimental procedure is compared to optical heterodyne detection Raman-induced Kerr effect spectroscopy (OHD-RIKES) and the data is compared with standard frequency-domain measurements.

AB - The stimulation and detection of both the A - and E -symmetry Raman lines in α-quartz using ultrafast impulsive stimulated Raman scattering is presented. Using a flexible experimental set-up, each nuclear oscillatory mode is selected and analysed in the time domain separately. The mode selection is made possible with optical summing of the fields involved to reduce noise and assure accurate synchronization. The experimental procedure is compared to optical heterodyne detection Raman-induced Kerr effect spectroscopy (OHD-RIKES) and the data is compared with standard frequency-domain measurements.

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Polarization-dependent detection of impulsive stimulated Raman scattering in α-quartz

Abstract

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